Hygroscopic properties and extinction of aerosol particles at ambient relative humidity in South-Eastern China

H. Eichler; Y. F. Cheng; W. Birmili; A. Nowak; A. Wiedensohler; E. Brüggemann; T. Gnauk; H. Herrmann; D. Althausen; A. Ansmann; R. Engelmann; Matthias Tesche; M. Wendisch; Y. H. Zhang; M. Hu; S. Liu; L. M. Zeng

doi:10.1016/j.atmosenv.2008.05.007

Hygroscopic properties and extinction of aerosol particles at ambient relative humidity in South-Eastern China

H. Eichler, Y. F. Cheng, W. Birmili, A. Nowak, A. Wiedensohler, E. Brüggemann, T. Gnauk, H. Herrmann, D. Althausen, A. Ansmann, R. Engelmann, Matthias Tesche, M. Wendisch, Y. H. Zhang, M. Hu, S. Liu, L. M. Zeng

Research output: Contribution to journal › Article › peer-review

64 Citations (Scopus)

Abstract

During the "Program of Regional Integrated Experiments of Air Quality over Pearl River Delta 2004 (PRIDE-PRD2004)" hygroscopic properties of particles in the diameter range 22 nm to 10 μ m were determined. For that purpose, a Humidifying Differential Mobility Particle Sizer (H-DMPS) and a Micro-Orifice Uniform Deposition Impactor (MOUDI) were operated. The derived size-dependent particle hygroscopic growth factors were interpolated to ambient relative humidity (RH) and used to calculate the particle number size distributions (PNSDs) at ambient conditions. A comparison between the modeled particle extinction coefficients (σ_{ext, Mie}) and those observed with a Raman lidar was made. It is shown that the particle extinction coefficient (σ_ext) at ambient RH can be properly estimated with Mie-model calculations based on the in situ physico-chemical measurements of dry and humidified PNSD and chemical composition.

Original language	English
Pages (from-to)	6321-6334
Number of pages	14
Journal	Atmospheric Environment
Volume	42
Issue number	25
DOIs	https://doi.org/10.1016/j.atmosenv.2008.05.007
Publication status	Published - Aug 2008

Keywords

Descriptive hygroscopic growth factor
H-DMPS
Hygroscopicity
Particle extinction coefficient
PRD

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10.1016/j.atmosenv.2008.05.007

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Eichler, H., Cheng, Y. F., Birmili, W., Nowak, A., Wiedensohler, A., Brüggemann, E., Gnauk, T., Herrmann, H., Althausen, D., Ansmann, A., Engelmann, R., Tesche, M., Wendisch, M., Zhang, Y. H., Hu, M., Liu, S., & Zeng, L. M. (2008). Hygroscopic properties and extinction of aerosol particles at ambient relative humidity in South-Eastern China. Atmospheric Environment, 42(25), 6321-6334. https://doi.org/10.1016/j.atmosenv.2008.05.007

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title = "Hygroscopic properties and extinction of aerosol particles at ambient relative humidity in South-Eastern China",

abstract = "During the {"}Program of Regional Integrated Experiments of Air Quality over Pearl River Delta 2004 (PRIDE-PRD2004){"} hygroscopic properties of particles in the diameter range 22 nm to 10 μ m were determined. For that purpose, a Humidifying Differential Mobility Particle Sizer (H-DMPS) and a Micro-Orifice Uniform Deposition Impactor (MOUDI) were operated. The derived size-dependent particle hygroscopic growth factors were interpolated to ambient relative humidity (RH) and used to calculate the particle number size distributions (PNSDs) at ambient conditions. A comparison between the modeled particle extinction coefficients (σext, Mie) and those observed with a Raman lidar was made. It is shown that the particle extinction coefficient (σext) at ambient RH can be properly estimated with Mie-model calculations based on the in situ physico-chemical measurements of dry and humidified PNSD and chemical composition.",

keywords = "Descriptive hygroscopic growth factor, H-DMPS, Hygroscopicity, Particle extinction coefficient, PRD",

author = "H. Eichler and Cheng, {Y. F.} and W. Birmili and A. Nowak and A. Wiedensohler and E. Br{\"u}ggemann and T. Gnauk and H. Herrmann and D. Althausen and A. Ansmann and R. Engelmann and Matthias Tesche and M. Wendisch and Zhang, {Y. H.} and M. Hu and S. Liu and Zeng, {L. M.}",

year = "2008",

month = aug,

doi = "10.1016/j.atmosenv.2008.05.007",

language = "English",

volume = "42",

pages = "6321--6334",

journal = "Atmospheric Environment",

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Eichler, H, Cheng, YF, Birmili, W, Nowak, A, Wiedensohler, A, Brüggemann, E, Gnauk, T, Herrmann, H, Althausen, D, Ansmann, A, Engelmann, R, Tesche, M, Wendisch, M, Zhang, YH, Hu, M, Liu, S & Zeng, LM 2008, 'Hygroscopic properties and extinction of aerosol particles at ambient relative humidity in South-Eastern China', Atmospheric Environment, vol. 42, no. 25, pp. 6321-6334. https://doi.org/10.1016/j.atmosenv.2008.05.007

TY - JOUR

T1 - Hygroscopic properties and extinction of aerosol particles at ambient relative humidity in South-Eastern China

AU - Eichler, H.

AU - Cheng, Y. F.

AU - Birmili, W.

AU - Nowak, A.

AU - Wiedensohler, A.

AU - Brüggemann, E.

AU - Gnauk, T.

AU - Herrmann, H.

AU - Althausen, D.

AU - Ansmann, A.

AU - Engelmann, R.

AU - Tesche, Matthias

AU - Wendisch, M.

AU - Zhang, Y. H.

AU - Hu, M.

AU - Liu, S.

AU - Zeng, L. M.

PY - 2008/8

Y1 - 2008/8

N2 - During the "Program of Regional Integrated Experiments of Air Quality over Pearl River Delta 2004 (PRIDE-PRD2004)" hygroscopic properties of particles in the diameter range 22 nm to 10 μ m were determined. For that purpose, a Humidifying Differential Mobility Particle Sizer (H-DMPS) and a Micro-Orifice Uniform Deposition Impactor (MOUDI) were operated. The derived size-dependent particle hygroscopic growth factors were interpolated to ambient relative humidity (RH) and used to calculate the particle number size distributions (PNSDs) at ambient conditions. A comparison between the modeled particle extinction coefficients (σext, Mie) and those observed with a Raman lidar was made. It is shown that the particle extinction coefficient (σext) at ambient RH can be properly estimated with Mie-model calculations based on the in situ physico-chemical measurements of dry and humidified PNSD and chemical composition.

AB - During the "Program of Regional Integrated Experiments of Air Quality over Pearl River Delta 2004 (PRIDE-PRD2004)" hygroscopic properties of particles in the diameter range 22 nm to 10 μ m were determined. For that purpose, a Humidifying Differential Mobility Particle Sizer (H-DMPS) and a Micro-Orifice Uniform Deposition Impactor (MOUDI) were operated. The derived size-dependent particle hygroscopic growth factors were interpolated to ambient relative humidity (RH) and used to calculate the particle number size distributions (PNSDs) at ambient conditions. A comparison between the modeled particle extinction coefficients (σext, Mie) and those observed with a Raman lidar was made. It is shown that the particle extinction coefficient (σext) at ambient RH can be properly estimated with Mie-model calculations based on the in situ physico-chemical measurements of dry and humidified PNSD and chemical composition.

KW - Descriptive hygroscopic growth factor

KW - H-DMPS

KW - Hygroscopicity

KW - Particle extinction coefficient

KW - PRD

U2 - 10.1016/j.atmosenv.2008.05.007

DO - 10.1016/j.atmosenv.2008.05.007

M3 - Article

AN - SCOPUS:49349110233

SN - 1352-2310

VL - 42

SP - 6321

EP - 6334

JO - Atmospheric Environment

JF - Atmospheric Environment

IS - 25

ER -

Hygroscopic properties and extinction of aerosol particles at ambient relative humidity in South-Eastern China

Abstract

Keywords

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